You should start seeing artifacts (little anomolies) on the screen if you've pushed it too far. I went to 400mhz on the memory on a GF2 GTS 64mb, and it was a bit too much. I dropped it down to 385mhz, and it was stable for awhile, but then started getting some artifacts. So, I just went back to the factory of 365mhz, and resigned that it's set about as good as it's gonna get and be rock solid stable.
bloom is right on the price issues, you should wait until the next gen comes out as it should put prices down, sorry I didn't point that out!

He's also right in that your current system might not take advantage of the better card (honestly, I dunno where the CPU bottleneck point on GF2 vs GF3 would be. I think I saw an article on that recently, I'll look for it.) However, if you're possibly planning to upgrade the CPU/mobo in the relatively near future, you could grow into the better card. Otherwise you'd upgrade to a significantly good processor and your vid card that you just upgraded is your bottleneck again. Yet another thing to worry about when upgrading components. lol.
Found the article at Toms Hardware that had CPU scaling in it.
The article (also posted in another thread) Click on CPU scaling to jump right to that section. Test setup will give you info on the 3 systems they used. If you look at the 800mhz system in Quake and then in Max Payne, you can see that it depends on the application as to whether you're going to get an increase from the GF2 Ti vs the GF3 Ti 200.
Also, this is just one article and one site's review. Your mileage may vary.
